>>2750522
>e. I want to get back to Rio by bus after that.
Why? Long journey.
3 full days in Foz is enough. 1 for argentinian side, one for brazilian and bird park and another for shitty Ciudad del este, the dam and triple border monument.... 4 is more comfortable.
From Foz you would be heading north to Rio. Only one state inbetween, São Paulo, at southeastern region (like Rio). Perhaps go a bit southeast to Florianopolis, nice city. Curitiba, Parana's capital is nice big city by brazilian standards, liveable, but not really touristic. Ilhabela is nice but a bit of a detour.
I'd just head to either Paraty, nice colonial town in Rio de Janeiro's state seaside or to Angra dos Reis (Ilha Grande). Paraty has both the town itself and the nature (the "fjord", some islands) and Ilha Grande and sorroundings is just nature but beautiful, more than 200 islands, 1000 beaches.

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Iguaçu Falls and south of Brazil